# A review on mathematical models for estimating indoor radon concentrations

- Ji Hyun Park
^{1}, - Dae Ryong Kang
^{2}and - Jinheum Kim
^{3}Email author

**28**:7

https://doi.org/10.1186/s40557-016-0091-6

© Park et al. 2016

**Received: **18 January 2016

**Accepted: **18 February 2016

**Published: **25 February 2016

## Abstract

Radiation from natural sources is one of causes of the environmental diseases. Radon is the leading environmental cause of lung cancer next to smoking. To investigate the relationship between indoor radon concentrations and lung cancer, researchers must be able to estimate an individual’s cumulative level of indoor radon exposure and to do so, one must first be able to assess indoor radon concentrations. In this article, we outline factors affecting indoor radon concentrations and review related mathematical models based on the mass balance equation and the differential equations. Furthermore, we suggest the necessities of applying time-dependent functions for indoor radon concentrations and developing stochastic models.

### Keywords

Mathematical model Indoor concentration Radon entry Exposure## Background

Exposure to radiation from natural sources leads to various environmental diseases. Radon, which is the primary constituent of natural radiation [1], is the leading environmental cause of lung cancer next to smoking [2]. Studies in Europe, the United States, Canada, and China have effectively shown a relationship between indoor radon concentrations and lung cancer [3].

*t*

_{1}to

*t*

_{2}, an individual’s cumulative level of indoor radon exposure can be defined as

*C*

_{ i }(

*t*) is the indoor radon concentration (Bq/m

^{3}) at time

*t*and

*V*is the volume of the building of interest (m

^{3}).

*C*

_{ i }(

*t*) can be affected by several factors: The United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR) reported that the 56 % of the radon that enters into a building comes from the soil, 21 % from building material (BM), 20 % from outdoor air, 2 % from a building’s water supply, and 1 % from natural gas [4]. As shown in Fig. 1 (see [5, 6] for more details), radon in the soil permeates a building: diffusive and advective flow; radon from BM diffuses into buildings. A building’s water supply and natural gas are also sources that introduce radon into a building, although that from natural gas is not generally considered because it is difficult to measure and contributes to only very small concentrations. Additionally, indoor radon concentrations can also vary as a result of air exchange between indoor and outdoor air.

There had been several studies to estimate the indoor radon concentrations with mathematical models. Ramola et al. [7] estimated the indoor radon concentration using a mathematical model based on the radon flux in soil and groundwater. Arvela et al. [8] calculated the indoor radon concentrations with a mathematical model which considers diffusion from soil and BM sources and air exchange simultaneously. These calculations have been compared with the measured variations of Finnish dwellings. Font [5] and Font and Baixeras [6] developed a generic and dynamic model of Radon Generation, Entry, and Accumulation indoors (RAGENA) which describes all the known sources including soil, BM, and water, and this model has been adapted to a Mediterranean climate house and Swedish house [9, 10]. Mathematical models for estimating indoor radon concentrations in high-rise buildings have been conducted by Man and Yeung [11] and Shaikh et al. [12]. These models included the contributions from BM and outdoor air. Moreover, model of indoor radon concentration in thermal spas was developed by Vogiannis and Nikolopoulos [13].

Notation

Symbol | Unit | Description |
---|---|---|

| Bq/m | Radon concentration in building material (BM) |

| Bq/m | Indoor radon concentration |

| Bq/m | Radon concentration of outdoor air |

| Bq/m | Radon concentration in soil |

| Bq/m | Radon concentration in water supply |

| Bq/(m | Total radon flux from soil into building |

| m/(s · Pa) | Advection transfer coefficient of soil |

| m/s | Diffusion transfer coefficient of BM |

| m/s | Diffusion transfer coefficient of soil |

| m | Air current from compartment |

| m | Indoor surface area of radon containing BM |

| m | Building area towards ground |

| dimensionless | Radon transfer efficiency of water supply |

| m | Use rate of water |

V | m | Volume of the indoor |

| Pa | Soil-indoor pressure difference |

λ | 1/s | Radon decay constant |

| 1/s | Ventilation rate |

## Review

According to the above, changes in indoor radon concentrations are affected by the sources of radon entry, building ventilation (radon exchange), and decay reaction. First, we introduce a model for assessing indoor radon concentrations attributed to the three main sources of radon entry (soil, BM, and water) and decay reaction.

### Radon entry and decay reaction

#### Soil

*F*

_{ s }in Equation (abbre. Eq.) (1) can be calculated as

Although radon from groundwater contributes very little to indoor radon, it can constitute an important source in specific instances; the total radon flux from the ground, considering both radon in soil and groundwater, can be found in Ramola et al. [9]. In the meantime, Font [5] and Font and Baixeras [6] suggested evaluating total radon flux from the soil into the building *F*
_{
s
} differently: the soil can be divided into two compartments, disturbed soil (DS, the volume of soil underneath a building from which radon can reach the basement of the building by diffusion and pressure driven flow) and undisturbed soil (US, the soil attached to the DS that is not influenced by the presence of the building). The radon concentrations in the US and in the DS are described in [5, 6]. However, for simplicity, throughout this article we develop a model using a total radon flux into the building that consider only DS, namely *F*
_{
s
} in Eq. (2).

#### Building material

#### Water for living

(see [5, 6, 13] for more details).

where *dC*
_{
i
} = *C*
_{
i
}(*t* + *dt*) − *C*
_{
i
}(*t*) and *dt* denotes an infinitesimal time.

### Radon exchange

#### Ventilation between indoor and outdoor air

where *λ*
_{
v
}(*C*
_{
i
} − *C*
_{
o
}) describes the radon exchange between indoor and outdoor air [5, 6, 9–16]. In Eq. (7), one may assume that *λ* = 0 because *λ* is relatively smaller than *λ*
_{
v
}.

#### Ventilation among the compartments

*N*compartments for more realistic models. In this case, from Eq. (7) the model for indoor radon concentration of

*i*th compartment is derived as

where the last term describes the radon exchange between compartments *i* and *j* [5, 6].

Summary of references reviewed in this article

Author(s) | Year | Factor | Application | Method | |||
---|---|---|---|---|---|---|---|

Soil | BM | Water | Vent. | ||||

Kusuda et al. [16] | 1980 | - | - | - | ○ | Sample calculations | N.S. |

Capra et al. [14] | 1994 | - | - | - | ○ | An environmental chamber | N.S. |

Ramola et al. [9] | 2011 | ○ | - | - | ○ | Budhakedar area of Garhwal Himalaya in summer and winter | N.S.S. |

Man and Yeung [11] | 1999 | - | ○ | - | ○ | Newly constructed, uninhabited high-rise buildings in Hong Kong | N.S.S. |

Shaikh et al. [12] | 2003 | - | ○ | - | ○ | A multi-storey building in Mumbai, India over four seasons | N.S.S. |

Vogiannis and Nikolopoulos [13] | 2008 | - | - | ○ | ○ | Thermal spas in Greece | N.M. |

Jelle [15] | 2012 | ○ | ○ | - | ○ | Sample calculations | N.S.S. |

Arvela et al. [10] | 1988 | ○ | ○ | - | ○ | Finnish dwellings in summer and winter | N.S.S. |

Font [5] | 1997 | ○ | ○ | ○ | ○ | Mediterranean climate house and Swedish house | N.M. |

Font and Baixeras [6] | 2003 |

## Conclusions

Mathematical models for estimating indoor radon concentrations provide not only a method of assessment but also an understanding between parameters that govern indoor radon levels. In order to estimate an individual’s cumulative indoor radon exposure, assessing indoor radon concentrations is necessary. To do so, one should seek to understand the mechanisms of radon entry and exchange in relation to side-specific surroundings and characteristics of a building. Accordingly, resultant models in consideration of said characteristics may be simpler than Eq. (8) or may necessitate additional research on factors of indoor radon concentrations (e.g., age of the BM and relative humidity).

Most of the models reviewed in this article utilized solutions at a steady state and considered parameters to be constant in order to estimate indoor radon concentrations. Such approaches are often adequate, as a steady state is rarely attained in actual buildings because of time-dependent factors (e.g., air exchange rates, which change with atmospheric conditions). For this reason, time-dependent solutions may be more accurate than steady state solutions in assessment of actual building conditions. Additionally, all of the models included in this review considered only deterministic models. However, a stochastic model designed to account for unrecognized factors and noise-corrupted measurements may offer better approximation of indoor radon levels.

## Declarations

### Acknowledgements

This subject is supported by Korea Ministry of Environment (MOE) as “the Environmental Health Action Program” (Grant Number 2015001350002).

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## Authors’ Affiliations

## References

- World Health Organization. Ionizing radiation in our environment. Geneva: World health; 2011. http://www.who.int/ionizing_radiation/env/en. Accessed 17 Dec 2011.Google Scholar
- US Environmental Protection Agency (EPA). News Releases – Air. EPA Joins Global Call-to-Action on Radon Cancer Dangers; 2009. http://yosemite.epa.gov/opa/admpress.nsf/6424ac1caa800aab85257359003f5337/8575b629701ce77b85257638005ef218!OpenDocument. Accessed 23 Apr 2010.
- World Health Organization. WHO handbook on indoor radon: a public health perspective. Geneva: World Health Organization; 2009. http://whqlibdoc.who.int/publications/2009/9789241547673_eng.pdf. Accessed 2 Nov 2014.Google Scholar
- United Nations Scientific Committee on the Effects of Atomic Radiation. UNSCEAR Report 1993: Sources and effects of ionizing radiation. New York: United Nations; 1993.Google Scholar
- Font Ll, Radon generation, entry and accumulation indoors. Ph.D. Thesis. Universitat Autònoma de Barcelona, Spain. 1997:138.Google Scholar
- Ll F, Baixeras C. The RAGENA dynamic model of radon generation, entry and accumulation indoors. Sci Total Environ. 2003;307(1):55–69.Google Scholar
- Font LI, Baixeras C, Domingo C, Fernández F. Experimental and theoretical study of radon levels and entry mechanisms in a Mediterranean climate house. Radiat Meas. 1999;31(1):277–82.View ArticleGoogle Scholar
- Ll F, Baixeras C, Jönsson G, Enge W, Ghose R. Application of a radon model to explain indoor radon levels in a Swedish house. Radiat Meas. 1999;31(1):359–62.Google Scholar
- Ramola RC, Prasad G, Gusain GS. Estimation of indoor radon concentration based on radon flux from soil and groundwater. Appl Radiat Isot. 2011;69(9):1318–21.View ArticlePubMedGoogle Scholar
- Arvela H, Voutilainen A, Mäkeläinen I, Castrén O, Winqvist K. Comparison of predicted and measured variations of indoor radon concentration. Radiat Prot Dosimetry. 1988;24(1–4):231–5.Google Scholar
- Man CK, Yeung HS. Modelling and measuring the indoor radon concentrations in high-rise buildings in Hong Kong. Appl Radiat Isot. 1999;50(6):1131–5.View ArticlePubMedGoogle Scholar
- Shaikh AN, Ramachandran TV, Vinod KA. Monitoring and modelling of indoor radon concentrations in a multi-storey building at Mumbai, India. J Environ Radioact. 2003;67(1):15–26.View ArticlePubMedGoogle Scholar
- Vogiannis E, Nikolopoulos D. Modelling of radon concentration peaks in thermal spas. application to Polichnitos and Eftalou spas (Lesvos Island—Greece). Sci Total Environ. 2008;405(1):36–44.View ArticlePubMedGoogle Scholar
- Capra D, Silibello C, Queirazza G. Influence of ventilation rate on indoor radon concentration in a test chamber. J Environ Radioact. 1994;24(3):205–15.View ArticleGoogle Scholar
- Jelle BP. Development of a model for radon concentration in indoor air. Sci Total Environ. 2012;416:343–50.View ArticlePubMedGoogle Scholar
- Kusuda T, Silberstein S, Mcnall PE. Modeling of radon and its daughter concentrations in ventilated spaces. J Air Pollut Control Assoc. 1980;30(11):1201–7.View ArticleGoogle Scholar